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Thus, the triplet excitons, which play a primary role in the photo-oxidation process, can be quenched by overlapping the energy level of the triplet state with the optical absorption of 402 Polymer nanocomposites metal nanoparticles and by increasing the contact area between the polymer and the metal nanoparticles. The gold nanoparticles dispersed in the PDOF solution were spin cast on glass substrates. In addition, the PL peak wavelength was not affected by the interaction between the polymer and the gold nano- particles. In general, excited chromophores can return to the ground state through a number of pathways involving both intermolecular and intramolecular interactions. While the system changes the state, both physical and chemical changes may occur. Two major chemical degradation processes, oxidation and cross-linking, can change the chemical structure of the original chromophore, 15. 0 Optical absorption of gold nanoparticles dispersed in chlorobenzenesolution. A TEM image of the gold nanoparticle is shown in the inset. Reprintedwith permission from J. . Park et al. Rapid Commun. 24, 331 (2003). Filled polymer nanocomposites and functionalized nanoparticles 403 resulting in increased non-radiative relaxation rates. Regarding the chemical route, Bliznyuk et al. 1 reported that oxidation of a polymer leads to the formation of carbonyl-containing species, which quench fluorescence. Because photo-induced oxidation of conjugated polymers begins with the formation of singlet oxygen via the energy transfer from long-lived triplet excitons, the triplet 15. 1 Optical absorption and PL spectra as a function of gold nanoparticlesvolume fraction. Reprinted with permission from J.

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